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• W1640248156 abstract "We present a Kadanoff-Baym formalism to study time-dependent phenomena for systems of interacting electrons and phonons in the framework of many-body perturbation theory. The formalism takes correctly into account effects of the initial preparation of an equilibrium state and allows for an explicit time-dependence of both the electronic and phononic degrees of freedom. The method is applied to investigate the charge neutral and non-neutral excitation spectra of a homogeneous, two-site, two-electron Holstein model. This is an extension of a previous study of the ground state properties in the Hartree (H), partially self-consistent Born (Gd) and fully self-consistent Born (GD) approximations published in Säkkinen et al. [J. Chem. Phys. 143, 234101 (2015)]. Here, the homogeneous ground state solution is shown to become unstable for a sufficiently strong interaction while a symmetry-broken ground state solution is shown to be stable in the Hartree approximation. Signatures of this instability are observed for the partially self-consistent Born approximation but are not found for the fully self-consistent Born approximation. By understanding the stability properties, we are able to study the linear response regime by calculating the density-density response function by time-propagation. This amounts to a solution of the Bethe-Salpeter equation with a sophisticated kernel. The results indicate that none of the approximations is able to describe the response function during or beyond the bipolaronic crossover for the parameters investigated. Overall, we provide an extensive discussion on when the approximations are valid and how they fail to describe the studied exact properties of the chosen model system." @default.
• W1640248156 created "2016-06-24" @default.
• W1640248156 creator A5006348044 @default.
• W1640248156 creator A5040317071 @default.
• W1640248156 creator A5065530872 @default.
• W1640248156 creator A5066773063 @default.
• W1640248156 date "2015-12-15" @default.
• W1640248156 modified "2023-09-29" @default.
• W1640248156 title "Many-body Green’s function theory for electron-phonon interactions: The Kadanoff-Baym approach to spectral properties of the Holstein dimer" @default.
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• W1640248156 doi "https://doi.org/10.1063/1.4936143" @default.
• W1640248156 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26696041" @default.
• W1640248156 hasPublicationYear "2015" @default.
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