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- W1644366838 abstract "Photoemission spectroscopy has been used to study a number of aspects of the mixed valent state (corresponding to non-integral 4f occupation) in rare earth systems. Deep core photoemission (e.g., from 3d or 4d levels) allows the measurement of the 4f occupancy and surface valence shifts, and, as well, the indirect measurement of the effect of solid state environment on the energy of hybridization between 4f electrons and conduction electrons. 4f-Derived photemission has been used to study surface valence and chemical shifts and to infer the nature of the mixed valent ground state. A combination of 4f-derived photoemission and add-electron spectroscopy provides a measurement of the 4f Coulomb correlation energy, an important parameter in the mixed valent problem. A review of these approaches is presented, with emphasis on Ce-based systems, whose behavior falls outside the usual description of 4f-unstable systems. 35 references." @default.
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- W1644366838 date "1984-01-01" @default.
- W1644366838 modified "2023-09-27" @default.
- W1644366838 title "Photoemission studies of mixed valent systems" @default.
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