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• W1644723035 abstract "We report results of high-resolution measurements of the c*‐axis expansivity (αc*) at the charge-ordering (CO) transition for the quasi-1D (TMTTF)2X compounds with X=SbF6 and Br and make a comparison with previous results for the X=PF6 and AsF6 salts. For X=SbF6, due to the screening of the long-range Coulomb forces, a sharp λ-type anomaly is observed at TCO, which contrasts with the step-like mean-field anomaly at TCO for PF6 and AsF6, where CO occurs in the Mott–Hubbard charge-localized regime. For the latter two salts, a negative contribution to αc* is observed above TCO. This feature is assigned to the anions’ rigid-unit modes, which become inactive for T<TCO. Our αc* results for the X=Br salt, where such rigid-unit modes are absent, reveal no traces of such negative contribution, confirming the model based on the anions’ rigid-unit modes for the X=PF6 and AsF6 salts." @default.
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• W1644723035 date "2010-06-01" @default.
• W1644723035 modified "2023-09-30" @default.
• W1644723035 title "Exploring the charge-ordering transition in via thermal expansion measurements" @default.
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• W1644723035 doi "https://doi.org/10.1016/j.physb.2009.12.022" @default.
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