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• W1648754734 abstract "Time-resolved coherent anti-Stokes Raman scattering, with a resolution of 20 fs, is used to prepare a broadband vibrational superposition on the ground electronic state of I2 isolated in solid Kr. The coherent evolution of a packet consisting of ν=1–6 is monitored for as many as 1000 periods, allowing a precise analysis of the material response and radiation coherence. The molecular vibrations are characterized by ωe=211.330(2) cm−1, ωexe=0.6523(6) cm−1, ωeye=2.9(1)×10−3 cm−1; the dephasing rates at 32 K range from 110 ps for ν=1 to 34 ps for ν=6, with ν dependence: γ(ν)=8.5×10−3+4.9×10−4ν2+2.1×10−6ν4 ps−1. The signal amplitude is also modulated at ωq=41.56(3) cm−1; which can be interpreted as coupling between the molecule and a local mode. The surprising implication is that this resonant local mode is decoupled from the lattice phonons, a finding that cannot be rationalized based on a normal-mode analysis." @default.
• W1648754734 created "2016-06-24" @default.
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• W1648754734 date "2003-12-23" @default.
• W1648754734 modified "2023-09-23" @default.
• W1648754734 title "Vibrational coherence of I2 in solid Kr" @default.
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• W1648754734 doi "https://doi.org/10.1063/1.1630567" @default.
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