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- W1649118966 abstract "We study the chemisorption of hydrogen at the surface and interface of Pd/W(110) and Pd/Ta(110) systems. To this goal a self-consistent tight-binding scheme is employed with repulsive interactions between atoms fitted to experimental data. For an epitaxial Pd overlayer the hydrogen chemisorption energy is essentially lower than at the Pd(111) surface. This conclusion can be partly modified by possible structural changes in the overlayer. Correlation of the surface reactivity with the electronic structure at the Fermi level and with core-level shifts is discussed. The hydrogen absorption below the Pd overlayer is rather likely especially for the Ta substrate." @default.
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- W1649118966 date "1995-07-01" @default.
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- W1649118966 title "Hydrogen chemisorption at the surface and interface of Pd/W(110) and Pd/Ta(110)" @default.
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- W1649118966 doi "https://doi.org/10.1016/0039-6028(95)00211-1" @default.
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