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- W1653120073 abstract "Here we study the polaronic transport through molecules weakly connected to metallic electrodes in the nonlinear response regime. Molecule itself is treated as a quantum dot with discrete energy levels, its connection to the electrodes is described within the wide-band approximation, while the charging is incorporated by means of the self-consistent potential. Nonperturbative computational scheme, used in this work, is based on the Green's function theory within the framework of mapping technique (GFT-MT). This method transforms the many-body electron-phonon interaction problem into a one-body multi-channel single-electron scattering problem with occupation of polaron levels calculated in the self-consistent way. In particular, three different phenomena as a result of charging in polaronic transport via discrete quantum states are discussed in detail: the suppression of the current at higher voltages, negative differential resistance (NDR effect), and rectification." @default.
- W1653120073 created "2016-06-24" @default.
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- W1653120073 date "2006-02-08" @default.
- W1653120073 modified "2023-09-27" @default.
- W1653120073 title "Polaronic transport through molecular quantum dots: charging-induced NDR and rectifying behavior" @default.
- W1653120073 hasPublicationYear "2006" @default.
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