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- W1655084451 abstract "Optical and infrared spectra of dichromate ions in KCl, KBr, and KI matrices are reported. Optical spectra of Cr2O7−− consist of three absorption bands that are attributed to the electronic transitions A11(t16)→T21(t15t21); A11(t16)→E1(t15t21) or T21(t15t21); and A11(t16) →T21(t15e1) on the basis of molecular orbitals. Fine structure caused by coupled vibration-electronic transitions is observed in the A11(t16)→T21(t15e1) band. This fine structure further splits at low temperature (77°K) because of the symmetry lowering of the dichromate ion from Td to C3v. Infrared spectra show a number of lines. A model that assumes that the dichromate ion enters the lattice by replacing two halide ions with no charge compensating vacancy satisfactorily explains all the experimental results." @default.
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- W1655084451 date "1974-11-15" @default.
- W1655084451 modified "2023-09-29" @default.
- W1655084451 title "Electronic and vibrational spectra of Cr2O7−− ions in potassium halide matrices" @default.
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- W1655084451 doi "https://doi.org/10.1063/1.1681685" @default.
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