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• W1657337029 startingPage "237" @default.
• W1657337029 abstract "The study of vibrational and rotational relaxation in condensed phases has acquired a new dimension with the development of ultrashort laser pulses and the corresponding techniques for time-resolved optical measurements. Nowadays, infrared-as well as Raman-active transitions can be interrogated with shorter than picosecond (1 ps = 10-12 s) time-resolution using, e.g., infrared absorption saturation [1–4] and transient hole-burning [5] spectroscopy and a variety of time-resolved techniques of stimulated Raman scattering [6–10]. They are complementary to methods in which the linewidths and -shapes of the transitions are measured with high spectral resolution, such as in infrared absorption and persistent [11] hole-burning spectroscopy, and in spontaneous and stimulated Raman scattering [8] [12, Chap. 4]. In most optical investigations only the k ≃ o excitations can be investigated because of the small wavevector of the light and the requirement of wavevector conservation. The goal of these experiments is to acquire a detailed understanding of the relaxation mechanisms of the molecular excitations in solids, relating them to different microscopic effects which are specific for the system under study: anharmonic interactions, impurity scattering, compositional or structural disorder, etc…. Excellent reviews have been published during the past several years, covering the study of the relaxation of internal and external vibrational modes in molecular crystals, and its experimental methods [7, 13–16]." @default.
• W1657337029 created "2016-06-24" @default.
• W1657337029 creator A5016613720 @default.
• W1657337029 date "1993-01-01" @default.
• W1657337029 modified "2023-09-27" @default.
• W1657337029 title "Relaxation of Frenkel-Type Rotational and Vibrational Excitons in Diatomic Molecular Crystals" @default.
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• W1657337029 doi "https://doi.org/10.1007/978-1-4615-2954-5_6" @default.
• W1657337029 hasPublicationYear "1993" @default.
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