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• W1657601036 abstract "Laser-ablation of six different metal targets with concurrent deposition of neon/nitric oxide samples at 4 K produces metal independent absorptions that can be assigned to charged (NO)2 species. The sharp 1227.3 cm−1 band and weaker 1225.1 cm−1 absorption show the different isotopic frequency ratios observed for the argon matrix counterparts at 1221.0 and 1222.7 cm−1 for trans-(NO)2− and cis-(NO)2−, respectively. Strong 1619.0 and weaker 1424.1 cm−1 absorptions, also observed in previous experiments with discharged neon, are enhanced with CCl4 doping while the (NO)2− bands are diminished, which supports cation identifications. These cation bands reverse absorbance with yellow and near-infrared photolysis. We suggested that the 1619.0 cm−1 band corresponds to the (NO)2+ isomer made by direct photoionization of cis-(NO)2. The 1424.1 cm−1 absorption shares the extreme red photosensitivity found for thermal (NO)2+ ions. Accordingly, the 1424.1 cm−1 absorption is probably due to the trans isomer, more stable in the gas phase, based on high level calculations, and the 1619.0 cm−1 band arises from the more stable matrix-isolated cis isomer with a dipole moment, which is produced by the more favorable Franck–Condon photoionization of the cis-(NO)2 precursor." @default.
• W1657601036 created "2016-06-24" @default.
• W1657601036 creator A5029634322 @default.
• W1657601036 creator A5046362125 @default.
• W1657601036 date "1999-10-01" @default.
• W1657601036 modified "2023-10-14" @default.
• W1657601036 title "Infrared spectra of (NO)2− and (NO)2+ isomers trapped in solid neon" @default.
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• W1657601036 doi "https://doi.org/10.1063/1.479900" @default.
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