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• W1660451228 abstract "The vibrational energy relaxation in collisions between N2 molecules in the low- and medium-lying vibrationally excited levels was revisited using the semiclassical coupled-state method and the use of two different potential-energy surfaces having the same short-range potential recently determined from ab initio calculations but with different long-range interactions. Compared to the data reported in the classical work by Billing and Fisher [Chem. Phys. 43, 395 (1979)], the newly calculated vibration-to-translation rate constant K(1,0∣0,0) is in much better agreement with the available experimental data over a large temperature interval, from T=200K up to T=6000K. Nevertheless, as far as the vibration-to-translation exchanges are concerned, the lower-temperature regime remains quite critical in that the new rate constants do not completely account for the rate constant curvature suggested by the experiments for temperatures lower than T=500K. The dependence of the state-selected vibration-to-vibration rate constants, K(v,v−Δv∣0,1), both upon the vibrational quantum number v and the gas temperature are calculated. The substantial deviations from previously found behaviors could have major consequences for the vibrational kinetic modeling of N2-containing gas mixtures." @default.
• W1660451228 created "2016-06-24" @default.
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• W1660451228 date "2005-11-01" @default.
• W1660451228 modified "2023-10-18" @default.
• W1660451228 title "Vibrational energy transfer in N2–N2 collisions: A new semiclassical study" @default.
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• W1660451228 doi "https://doi.org/10.1063/1.2101445" @default.
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