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- W1660832023 abstract "We have investigated the magnetic properties of Ni2+ exchanged NaY zeolite by using a direct current magnetization technique. At T>5 K, the M vs H/T curves superimpose and these curves could be fitted well using a Langevin function with a log-normal distribution of moments. The mean spin-cluster moment has been found to be ∼3.3μB. The deviation from the superposition of the M vs H/T curves is observed at T<5 K indicating the building up of a spin-spin correlation between Ni clusters below 5 K. The zero-field-cooled and field-cooled magnetization curves show branching at low temperatures (T≤5 K) under low applied magnetic fields (H≤1 kOe) with a peak in the zero-field-cooled magnetization curves. A log-normal distribution of spin-freezing/blocking temperature has been observed with mean spin-freezing/blocking temperature ∼3.0 K. The peak temperature Tg decreases with increasing field and follows the de Almeida–Thouless (AT) line [1−Tg(H)/Tg(0)]∝H2/3. The extrapolation of the AT line gives the spin-freezing temperature Tg(0)≈3.29 K." @default.
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- W1660832023 date "2007-11-15" @default.
- W1660832023 modified "2023-10-17" @default.
- W1660832023 title "Magnetic properties of Ni2+ clusters in NaY zeolite" @default.
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- W1660832023 doi "https://doi.org/10.1063/1.2815624" @default.
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