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• W1665336327 abstract "Photoelectron imaging spectroscopy of (CS2)n−, n&gt;4, reveals a new state with an electron binding energy smaller than that of any of the corresponding CS2− and C2S4− states known to date. With support from ab initio calculations, two long-lived, metastable binding motifs with small electron binding energies are discussed for these clusters. The first is a solvent network permeating state, where the excess electron is delocalized over a number of linear CS2 molecules. The second is an excited B21 state of the core CS2− anion stabilized at a slightly bent geometry by the solvation interactions. Based on the observed solvation-induced shifts in binding energy, the second motif is favored." @default.
• W1665336327 created "2016-06-24" @default.
• W1665336327 creator A5014714039 @default.
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• W1665336327 date "2008-12-28" @default.
• W1665336327 modified "2023-09-27" @default.
• W1665336327 title "Electron binding motifs in the (CS2)n− (n&gt;4) cluster anions" @default.
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• W1665336327 doi "https://doi.org/10.1063/1.3046481" @default.
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