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- W166665018 abstract "We analyze the effect of relaxation process of wavepackets created in the electronic excited state on off-resonant two-dimensional Raman spectroscopy, employing the Brownian motion model with a nonequilibrium initial condition described by a displaced Gaussian wavepacket. We calculate three-time correlation functions of the excited state polarizability, which correspond to the fifth-order Raman signal in the excited state by using the Feynman’s path integral formalism. It is found that the fifth-order signal is sensitive to the initial position of the Gaussian wavepacket not only for the underdamped case but also for the overdamped case." @default.
- W166665018 created "2016-06-24" @default.
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- W166665018 date "2000-01-01" @default.
- W166665018 modified "2023-10-14" @default.
- W166665018 title "Dynamical stokes shift observed by two-dimensional Raman spectroscopy" @default.
- W166665018 doi "https://doi.org/10.1063/1.1302889" @default.
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