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• W1669710669 abstract "Laser-induced fluorescence and action spectroscopy experiments were performed to identify the origin of the Ar...I(2) continuum signals observed in and above the I(2) B-X spectral region. We have verified that these signals arise from transitions of the linear Ar...I(2) (X,v=0) complex. The data provides no evidence that the excited state complexes undergo a one-atom caging mechanism when prepared above the I(2)(B) dissociation limit, Ar...I(2) (B)*-->Ar+I+I*-->Ar+I(2)(B,v'). Instead, our results indicate that the continuum signals result from bound-free transitions of the linear Ar...I(2) X,v()=0) complex to the inner repulsive walls of numerous Ar+I(2)(B,v') intermolecular potentials. The bound-free continuum signal associated with transitions to each Ar+I(2)(B,v') potential spans an energy region >700 cm(-1). We have found that the continuum signals turn-on 250(2)cm(-1) above the corresponding I(2) B-X,v'-0 band origin, and this energy represents the binding energy of the linear Ar...I(2) (X,v=0) conformer, D(0) ()(L)=250(2)cm(-1)." @default.
• W1669710669 created "2016-06-24" @default.
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• W1669710669 date "2005-04-01" @default.
• W1669710669 modified "2023-09-29" @default.
• W1669710669 title "Observation of bound-free transitions of the linear Ar⋯I2(X,v″=) complex in and above the I2B-X spectral region" @default.
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• W1669710669 doi "https://doi.org/10.1063/1.1885001" @default.
• W1669710669 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/15847447" @default.
• W1669710669 hasPublicationYear "2005" @default.
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