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• W1671036714 abstract "Hydrogels that form via the self‐assembly of β‐hairpin peptides are studied for their potential use in biomedical applications. Multiple particle tracking microrheology and circular dichroism (CD) spectroscopy are used to study the gelation kinetics of four peptides that are engineered to exhibit responsive behavior to changes in environmental conditions. The peptides being compared differ in sequence by a point substitution of a single amino acid near the turn sequence, which predictably alters the energetics of the folding event. The principles of time‐cure superposition are used to rescale the mean‐squared displacement of probe particles onto master curves before and after the gel point. By analyzing the shift factors based on scaling relationships near the liquid‐solid transition, we are able to accurately determine both the gel time and critical exponents of the incipient gel. An empirical relationship is established between the rheologically‐defined gelation time and the onset of beta‐sheet formatio..." @default.
• W1671036714 created "2016-06-24" @default.
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• W1671036714 date "2008-01-01" @default.
• W1671036714 modified "2023-09-27" @default.
• W1671036714 title "Microrheology of Responsive Hydrogel Networks" @default.
• W1671036714 cites W1988147327 @default.
• W1671036714 doi "https://doi.org/10.1063/1.2964477" @default.
• W1671036714 hasPublicationYear "2008" @default.
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