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• W1673673571 abstract "Experimental values for the proton-spin-lattice relaxation time in CH4 and deuteroderivates and in CH4-CD4 mixtures are used to separate the different contributions to the relaxation rate. The results are compared with theoretical models. The spin-rotational interaction is shown to be the main contribution in the gas phase. The behaviour of the rotational correlation times are, even up to liquid densities best understood in terms of a kinetic model, using the so-called transient approximation. At liquid densities and low temperatures the intermolecular dipole-dipole interactions constitute the dominating mechanism. The experimental data for this contribution are in good agreement with theoretical predictions. Throughout the whole temperature and density region the intramolecular dipole-dipole interactions constitute only a small contribution. For the solid, rough estimates are obtained for the self-diffusion coefficient and the rotational correlation times and their activation energies." @default.
• W1673673571 created "2016-06-24" @default.
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• W1673673571 date "1971-02-01" @default.
• W1673673571 modified "2023-09-23" @default.
• W1673673571 title "Proton-spin-lattice relaxation and self-diffusion in methanes" @default.
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• W1673673571 doi "https://doi.org/10.1016/0031-8914(71)90049-8" @default.
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