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- W169336089 abstract "Gas generation, oxidation, corrosion, and other important phenomena accompanying the long-term storage of spent nuclear fuel (SNF) are highly affected by radiation-induced processes at oxide surfaces and interfaces. Oxides covering fuel rods and other surfaces, as well as oxide particles dispersed in the aqueous phase, can promote water radiolysis and decomposition. Surface-enhanced water radiolysis may accelerate oxidation, corrosion, and hydriding of Zircaloy, uranium, and other materials and may affect the amount of H{sub 2} and O{sub 2} produced during SNF storage. Mechanisms of surface-enhanced radiolysis are not well understood. Some proposed mechanisms are based on the transfer of energy initially deposited in the bulk of the oxide phase to the interface. This process depends on the oxide electronic structure and on the energetics and geometric structures of the adsorbed molecules. Typically, mobile electrons, holes, and excitons contribute to the enhancement. Their effective range is directly related to carrier mean free paths and excited state lifetimes. These parameters can be studied with a technique known as laser-stimulated luminescence (LSL). The authors present data on the gamma radiation-induced degradation of water at oxide particle/water interfaces and on time-resolved LSL measurements of ZrO{sub 2} recombination luminescence." @default.
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- W169336089 date "1999-07-01" @default.
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- W169336089 title "Radiation-induced processes at oxide surfaces and interfaces relevant to spent nuclear fuel storage" @default.
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