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- W1710901369 abstract "The study of artificial photosynthesis has been the subject of ongoing attention for many years now due to the need for sustainable energy resources. In natural photosynthesis, a light harvesting antenna system with a large optical cross-section (for example the LH2 complex) absorbs a photon that is funneled by energy transfer (ET) to the reaction centre. Excellent candidates to mimic the natural antenna system are molecules that efficiently absorb light and are able to transfer the captured energy to other parts of the molecule. Molecules based on Zn and free-base porphyrins are examples of compounds that can be used as models for the LH2 complex. This chapter investigates energy transfer between the Zn-porphyrin units in a sequence of dendrimers varying in size from 4 to 64 porphyrin units. Reference measurements are performed on the monomer, PlDl. In order to follow energy transfer within the dendrimers, the fluorescence anisotropy decay is analyzed. To determine the lifetime of the dendrimers, additional analysis of the kinetics measured at magic angle is performed." @default.
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- W1710901369 date "2004-01-01" @default.
- W1710901369 modified "2023-09-26" @default.
- W1710901369 title "Energy transfer in light-harvesting Zn porphyrin dendrimers" @default.
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- W1710901369 doi "https://doi.org/10.1016/b978-044451656-5/50096-7" @default.
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