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- W172345058 abstract "Time evolution of excited state population was studied theoretically for the system of two electronic levels coupled to two vibrational modes, which are also attached to a heat bath. In the excited state, the mutual coupling of the vibrational modes was included. It was demonstrated that excited state population relaxes faster if interacting vibrational mode dissipates its energy via vibrational mode of a smaller eigenfrequency. It was also demonstrated that fast component of excited state depopulation cannot be achieved via coherent mode-mode coupling, if the second mode is not directly coupled to the electronic inter-state transition.Key wordsexcited state relaxationelectron-vibrational interactionvibrational coherence" @default.
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- W172345058 date "2006-01-12" @default.
- W172345058 modified "2023-10-16" @default.
- W172345058 title "Vibration-Induced Excited State Decay" @default.
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