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- W1732499503 abstract "This work explores nucleation and epitaxy of graphene on crystalline Cu 2 O templates formed via self-assembly and surface reduction of Cu 2 O nanocrystallites on the cubic textured (100) orientation Cu (CTO-Cu) and polycrystalline Cu (poly-Cu) substrates, respectively. It has been found that the presence of sub-surface oxygen causes the reconstruction of Cu surface due to the formation of oriented Cu 2 O nanocrystallites at a low H 2 gas flow. Self-assembly of the Cu 2 O nanocrystallites into a textured surface template provides direct nucleation sites for graphene growth after the oxygen-sublattice on the template surface is reduced. The atomic Cu surface layer provides advantages of high graphene growth rate due to the catalytic role of Cu and in-plane alignment of graphene nuclei. It is particularly important that the Cu 2 O crystallites have predominantly (111) orientation aligned to each other in the plane of the (100) CTO-Cu substrates, which allows epitaxy of graphene with much lower defect density as compared to that in the poly-Cu case. Since Cu 2 O (111) templates may be developed on lattice matched (100) surfaces of other dielectric materials, this self-assembly approach provides a promising pathway for large-scale, transfer free graphene epitaxy on nonmetallic surfaces." @default.
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- W1732499503 date "2015-12-01" @default.
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- W1732499503 title "Direct graphene growth on (111) Cu2O templates with atomic Cu surface layer" @default.
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- W1732499503 doi "https://doi.org/10.1016/j.carbon.2015.08.071" @default.
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