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- W1781900019 abstract "We report the first high-resolution spectra for the out-of-plane librational vibration in the water dimer. Three vibrational subbands comprising a total of 188 transitions have been measured by diode laser spectroscopy near 500 cm(-1) and assigned to (H2O)2 libration-rotation-tunneling eigenstates. The band origin for the Ka = 1 subband is ~524 cm(-1). Librational excitation increases the interchange and bifurcation hydrogen bond rearrangement tunneling splittings by factors of 3-5 and 4-40, respectively. Analysis of the rotational constants obtained from a nonlinear least squares fit indicates that additional external perturbations to the energy levels are likely." @default.
- W1781900019 created "2016-06-24" @default.
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- W1781900019 date "2015-10-20" @default.
- W1781900019 modified "2023-10-18" @default.
- W1781900019 title "Far-infrared VRT spectroscopy of the water dimer: Characterization of the 20 <i>μ</i>m out-of-plane librational vibration" @default.
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- W1781900019 doi "https://doi.org/10.1063/1.4933116" @default.
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