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- W1785928710 abstract "We derive the moment generating function for photon emissions from a single molecule driven by laser excitation. The frequencies of the fluoresced photons are explicitly considered. Calculations are performed for the case of a two-level dye molecule, showing that measured photon statistics will display a strong and nonintuitive dependence on detector bandwidth. Moreover, it is demonstrated that the antibunching phenomenon, associated with negative values of Mandel's $Q$ parameter, results from correlations between photons with well separated frequencies." @default.
- W1785928710 created "2016-06-24" @default.
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- W1785928710 date "2009-01-09" @default.
- W1785928710 modified "2023-10-15" @default.
- W1785928710 title "Theory for Wavelength-Resolved Photon Emission Statistics in Single-Molecule Fluorescence Spectroscopy" @default.
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- W1785928710 doi "https://doi.org/10.1103/physrevlett.102.018303" @default.
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