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- W181520701 abstract "Shape selective catalysis by zeolites provides new insights into catalytic mechanisms as well as new capabilities for technology. Acidic zeolites provide a variety of highly selective aromatics transformations as well as new routes to their synthesis. Using ZSM-5 type catalysts, xylene isomerization is carried out with suppression of undesirable byproducts, and improved toluene disproportionation and ethyl-benzene synthesis processes have evolved. The kinetics and selectivities involved will be discussed. Furthermore, novel para-selective modes of alkylation or transalkylation reactions can be attained. They allow the synthesis of para-xylene, para-ethyl toluene, etc. Acidic ZSM-5 zeolites open up new routes to the synthesis of aromatics from a wide variety of non-aromatic molecules. In all these reactions, the formation and distribution of products is dominated by a few unifying mechanistic principles which follow classical carbenium ion theory. The active sites are the tetrahedral aluminum sites in the silicate framework. Most of the reactions are accomplished by a surprisingly small number of acidic sites." @default.
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- W181520701 date "1984-01-01" @default.
- W181520701 modified "2023-09-25" @default.
- W181520701 title "SHAPE-SELECTIVE CATALYSIS IN AROMATICS PROCESSING" @default.
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- W181520701 doi "https://doi.org/10.1016/b978-0-08-029249-6.50047-7" @default.
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