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- W181817400 abstract "NMR and $ensuremath{mu}mathrm{SR}$ relaxation measurements in the ${mathrm{Mn}}_{9}{({mathrm{C}}_{19}{mathrm{H}}_{15}{mathrm{N}}_{9}{mathrm{O}}_{2})}_{6}{({mathrm{ClO}}_{4})}_{6}.18{mathrm{H}}_{2}mathrm{O}({mathrm{Mn}}_{3ifmmodetimeselsetexttimesfi{}3})$ molecular grid are presented. The temperature dependence of the relaxation rates can be conveniently described by a single correlation time for the spin fluctuations at temperatures of the order of the exchange coupling among ${mathrm{Mn}}^{2+}$ ions. The inverse of the correlation time is observed to reach the MHz range at low temperature and its temperature dependence can be justified on the basis of a theoretical model where the electron spin fluctuations are driven by spin-phonon coupling. Finally, it is pointed out that the magnetic field dependence of the $ensuremath{mu}mathrm{SR}$ relaxation rate allows one to derive the Zeeman splitting of the low-energy spin levels." @default.
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- W181817400 date "2005-08-01" @default.
- W181817400 modified "2023-09-27" @default.
- W181817400 title "Low-energy spin excitations inMn3×3molecular nanomagnets" @default.
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- W181817400 doi "https://doi.org/10.1103/physrevb.72.064402" @default.
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