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- W1819091165 abstract "Catalytic asymmetric endo-selective [3+2] cycloaddition reactions of Schiff bases of α-aminophosphonates with olefins are described. While the efficient asymmetric synthesis of several phosphonate analogues of proline derivatives is important in bioorganic chemistry, a direct catalytic method to prepare optically active endo [3+2] cycloadducts of α-aminophosphonates with olefins has never been developed. We found for the first time that catalyst systems prepared from Group 11 metal amides with the (R)-FeSulphos ligand were effective for the asymmetric endo-selective [3+2] cycloaddition to afford the desired proline phosphonate analogues in high yields with high endo- and high enantioselectivities." @default.
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- W1819091165 date "2015-01-01" @default.
- W1819091165 modified "2023-10-16" @default.
- W1819091165 title "Catalytic asymmetric endo-selective [3+2] cycloaddition reactions of Schiff bases of α-aminophosphonates with olefins using chiral metal amides" @default.
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- W1819091165 doi "https://doi.org/10.1039/c5cc07066j" @default.
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