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- W1820090127 abstract "In this study, CO2 occlusion of K2CO3 was examined at different temperatures under moist conditions. The CO2 occlusion rate increased with increasing temperatures, whereas the saturated occlusion amount decreased. The highest occlusion amount (i.e. 6.48 mmol·g–1) was obtained at 313 K. Results of X-ray powder diffraction analysis showed that the formation of bicarbonate as a result of the K2CO3 decomposition with CO2 and H2O involved two reactions with K4H2(CO3)3·1.5H2O as an intermediate. It was determined that the lower saturated occlusion amount at higher temperatures originated from the exothermic property of the second reaction. Because the equilibrium constant for the bicarbonate formation is smaller at higher temperatures, the reaction does not proceed as quickly or efficiently according to Le Châtelier’s principle. Therefore, the CO2 occlusion of K2CO3 is suitable for the saturated occlusion amount at lower temperatures." @default.
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- W1820090127 date "2015-03-01" @default.
- W1820090127 modified "2023-09-27" @default.
- W1820090127 title "Temperature-Dependent Double-Step CO<sub>2</sub> Occlusion of K<sub>2</sub>CO<sub>3</sub> under Moist Conditions" @default.
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- W1820090127 doi "https://doi.org/10.1260/0263-6174.33.3.243" @default.
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