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- W1834221211 abstract "BaCe 0.9Nd 0.1O 3-α(BCN) ceramic is known to be an excellent high-temperature protonconductor and is a candidate electrolyte for use in solid oxide fuelcells, hydrogen or steam sensors and steam electrolysers. In this work,the chemical stability of BCN was investigated systematically by combiningXRD and DTA–TG techniques to study its processing compatibility andits feasibility in potential applications. It was found that above 1200°C, BCN reacted with alumina or zirconia, leading to the loss ofbarium and an excess of cerium. In cold water, both sintered BCN disks andpowder samples had very low solubility and did not hydrolyse, but theywere soluble in some mineral acids, especially in HCl with the liberationof Cl 2 . In boiling water, BCN pellets dissolved readily withdecomposition into CeO 2 and Ba(OH) 2 . In 1 atmCO 2 , BCN decomposed to form CeO 2 andBaCO 3 below 1200 °C during heating, but during cooling itwas stable above 1000 °C, possibly because BCN has different crystalstructures at low and high temperatures. At 600–1000 °C, BCNshowed a slight mass loss when exposed to a reducing atmosphere, and aslight mass gain in an oxidizing atmosphere. XRD results revealed that BCNdemonstrated chemical and structural stability in both reducing andoxidizing atmospheres." @default.
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- W1834221211 date "1997-01-01" @default.
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- W1834221211 title "Chemical stability study of BaCe0.9Nd0.1O3−α high-temperature proton-conducting ceramic" @default.
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- W1834221211 doi "https://doi.org/10.1039/a605377g" @default.
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