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- W1837332370 abstract "The demand for efficient chiral cyclopentadienyl ligands (Cp<sup>x</sup>) has increased significantly in recent years, partly because Cp*Rh(III) species have been developed as powerful catalysts for directed C–H functionalization reactions. However, a lack of suitable Cp<sup>x</sup> ligands has hampered the development of the corresponding enantioselective processes. We report expansions of the libraries of two generations of Cp<sup>x</sup> ligands and their corresponding rhodium(I) complexes. The potential of the rhodium complexes as catalysts was evaluated in enantioselective C–H functionalizations involving cyclizations across tethered aldehydes. The mild reaction conditions permit the syntheses of hydroxychromanes and phthalides in good yields and high enantioselectivities." @default.
- W1837332370 created "2016-06-24" @default.
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- W1837332370 date "2015-05-11" @default.
- W1837332370 modified "2023-10-01" @default.
- W1837332370 title "Chiral Cyclopentadienyl Ligands Enable a Rhodium(III)-Catalyzed Enantioselective Access to Hydroxychromanes and Phthalides" @default.
- W1837332370 cites W1543582093 @default.
- W1837332370 doi "https://doi.org/10.1055/s-0034-1380765" @default.
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