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- W183818285 abstract "The paper deals with the problem of surface effects at a fluid boundary produced by a step force field. A classical simple fluid with a locally placed field simulating a solid is considered. The specific surface -potential γ, the surface number density, and the Henry adsorption constant are determined. A surface cluster expansion (the expansion of the surface omega potential in powers of the activity) is obtained. This expansion is similar to the cluster expansion for the pressure in which the integrals of the Ursell factors are replaced by sums of the first-order moments of the Ursell factors over sectors or orthants. The contact theorem is extended to the case of a finite step field. It is found that the surface number density (its invariant part) is determined by the first-order moment of the pair Ursell function taken over the entire space. The high-and low-temperature limits are analyzed and are shown to be consistent with the previously obtained general results. Symmetry features of the solution with respect to permutation of the solid and fluid regions are established." @default.
- W183818285 created "2016-06-24" @default.
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- W183818285 date "2012-05-30" @default.
- W183818285 modified "2023-09-27" @default.
- W183818285 title "Statistical mechanics of fluids in a step potential" @default.
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