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- W1846870679 abstract "Recently, there has been much interest in the development and application of multidimensional coherent nonlinear femtosecond techniques for the study of electronic and vibrational dynamics of molecules. In such experiments, more than two laser pulses have been used and the combination of laser pulses in the sample creates a nonlinear polarization, which in turn radiates an electric field. The multiple laser pulses create wave packets of molecular states and establish a definite phase relationship (or coherence) between the different states. The laser pulses can create, manipulate, and probe this coherence, which is strongly dependent on the molecular structure, coupling mechanisms and the molecular environment, making the technique a potentially powerful method for studies of large molecules. This chapter reports the use of spectrally resolved two-colour three-pulse photon echoes to expand the information that can be obtained from time-resolved vibrational spectroscopy. The experiments allow the study of intramolecular dynamics and vibrational structure in both the ground and excited electronic states and demonstrate the potential of the technique for studying structural dynamics." @default.
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- W1846870679 date "2004-01-01" @default.
- W1846870679 modified "2023-09-27" @default.
- W1846870679 title "Spectrally resolved femtosecond two-colour three-pulse photon echoes for studies of molecular dynamics: influence of pulse wavelengths and pulse sequence" @default.
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- W1846870679 doi "https://doi.org/10.1016/b978-044451656-5/50020-7" @default.
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