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- W1848572169 abstract "In this study, we investigated the size, submicrometer-scale structure, and aggregation state of ZnS formed by sulfate-reducing bacteria (SRB) in a SRB-dominated biofilm growing on degraded wood in cold (T ~ 8 °C), circumneutral-pH (7.2−8.5) waters draining from an abandoned, carbonate-hosted Pb-Zn mine. High-resolution transmission electron microscope (HRTEM) data reveal that the earliest biologically induced precipitates are crystalline ZnS nanoparticles 1−5 nm in diameter. Although most nanocrystals have the sphalerite structure, nanocrystals of wurtzite are also present, consistent with a predicted size dependence for ZnS phase stability. Nearly all the nanocrystals are concentrated into 1−5 μm diameter spheroidal aggregates that display concentric banding patterns indicative of episodic precipitation and flocculation. Abundant disordered stacking sequences and faceted, porous crystalaggregate morphologies are consistent with aggregation-driven growth of ZnS nanocrystals prior to and/or during spheroid formation. Spheroids are typically coated by organic polymers or associated with microbial cellular surfaces, and are concentrated roughly into layers within the biofilm." @default.
- W1848572169 created "2016-06-24" @default.
- W1848572169 creator A5000954303 @default.
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- W1848572169 date "2004-07-01" @default.
- W1848572169 modified "2023-10-18" @default.
- W1848572169 title "Ultrastructure, aggregation-state, and crystal growth of biogenic nanocrystalline sphalerite and wurtzite" @default.
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- W1848572169 doi "https://doi.org/10.2138/am-2004-0704" @default.
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