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• W1850764185 abstract "This work represents the first report on the heat capacity of brookite TiO2, which was measured using a Quantum Design physical property measurement system (PPMS) in the temperature range of 2 K to 300 K. The experimental data were fitted using a series of theoretical functions for low temperatures (T < 15 K), orthogonal polynomials for mid temperatures (15 < T < 75 K), and a combination of Debye and Einstein functions for high temperatures (T > 75 K), from which the thermodynamic functions of brookite TiO2 were calculated. The standard molar entropy and molar enthalpy for brookite TiO2 at T = 298.15 K were determined to be 52.61 ± 0.53 J · K−1 · mol−1 and 9.03 ± 0.09 kJ · mol−1, respectively, leading to a Gibbs free energy of −6.65 ± 0.18 kJ · mol−1. Strikingly, this Gibbs free energy was found to be slightly less than those reported for rutile TiO2 (−6.377 kJ · mol−1) and anatase TiO2 (−6.198 kJ · mol−1) (Smith et al., 2009). Further data analyses demonstrated that the thermal stability of TiO2 polymorphs follows a sequence of anatase < rutile < brookite at T = 298.15 K." @default.
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• W1850764185 date "2016-02-01" @default.
• W1850764185 modified "2023-09-26" @default.
• W1850764185 title "Heat capacity and thermodynamic functions of brookite TiO 2" @default.
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• W1850764185 doi "https://doi.org/10.1016/j.jct.2015.09.018" @default.
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