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• W1865849968 abstract "We studied the dynamics in ultrathin subsurface layers of an amorphous polymer by the spectra of single fluorescent molecules embedded into the layer by vapor deposition and subsequent controlled diffusion to the desired depth in ≈0.5 nm steps. The spectral trails of single molecules were recorded at 4.5 K as a function of diffusion depth. In depths shallower than 20 nm, the spectral dynamics deviate from those deep in the bulk. Less than 5 nm deep, the linewidths increase rapidly, whereas the number of detected molecules decreases. No zero-phonon lines were observed closer than 0.5 nm to the polymer surface. Possible physical reasons of the observed phenomena are discussed." @default.
• W1865849968 created "2016-06-24" @default.
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• W1865849968 date "2015-01-01" @default.
• W1865849968 modified "2023-10-11" @default.
• W1865849968 title "Fluorescence microscopy and spectroscopy of subsurface layer dynamics of polymers with nanometer resolution in the axial direction" @default.
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• W1865849968 doi "https://doi.org/10.1039/c5fd00055f" @default.
• W1865849968 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26403863" @default.
• W1865849968 hasPublicationYear "2015" @default.
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