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• W1880580236 endingPage "013103" @default.
• W1880580236 startingPage "013103" @default.
• W1880580236 abstract "An ensemble inhomogeneity of non-spherical LaB6 nanoparticles dispersion has been analyzed with Mie theory to account for the observed broad plasmon band. LaB6 particle shape has been characterized using small-angle X-ray scattering (SAXS) and electron tomography (ET). SAXS scattering intensity is found to vary exponentially with exponent −3.10, indicating the particle shape of disk toward sphere. ET analysis disclosed dually grouped distribution of nanoparticle dispersion; one is large-sized at small aspect ratio and the other is small-sized with scattered high aspect ratio, reflecting the dual fragmentation modes during the milling process. Mie extinction calculations have been integrated for 100 000 particles of varying aspect ratio, which were produced randomly by using the Box-Muller method. The Mie integration method has produced a broad and smooth absorption band expanded towards low energy, in remarkable agreement with experimental profiles by assuming a SAXS- and ET-derived shape distribution, i.e., a majority of disks with a little incorporation of rods and spheres for the ensemble. The analysis envisages a high potential of LaB6 with further-increased visible transparency and plasmon peak upon controlled particle-shape and its distribution." @default.
• W1880580236 created "2016-06-24" @default.
• W1880580236 creator A5043506969 @default.
• W1880580236 creator A5048428374 @default.
• W1880580236 date "2015-07-07" @default.
• W1880580236 modified "2023-10-16" @default.
• W1880580236 title "Particle shape inhomogeneity and plasmon-band broadening of solar-control LaB₆ nanoparticles" @default.
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• W1880580236 doi "https://doi.org/10.1063/1.4923049" @default.
• W1880580236 hasPublicationYear "2015" @default.
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