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• W1887169285 abstract "Abstract Zeolites represent inorganic solid-state materials with porous structures of fascinating complexity. Recently, significant progress was made by reticular synthesis of related organic solid-state materials, such as metal-organic or covalent organic frameworks. Herein we go a step further and report the first example of a fluid honeycomb mimicking a zeolitic framework. In this unique self-assembled liquid crystalline structure, transverse-lying π-conjugated rod-like molecules form pentagonal channels, encircling larger octagonal channels, a structural motif also found in some zeolites. Additional bundles of coaxial molecules penetrate the centres of the larger channels, unreachable by chains attached to the honeycomb framework. This creates a unique fluid hybrid structure combining positive and negative anisotropies, providing the potential for tuning the directionality of anisotropic optical, electrical and magnetic properties. This work also demonstrates a new approach to complex soft-matter self-assembly, by using frustration between space filling and the entropic penalty of chain extension." @default.
• W1887169285 created "2016-06-24" @default.
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• W1887169285 date "2015-10-21" @default.
• W1887169285 modified "2023-10-14" @default.
• W1887169285 title "Zeolite-like liquid crystals" @default.
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• W1887169285 doi "https://doi.org/10.1038/ncomms9637" @default.
• W1887169285 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4639914" @default.
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