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- W1890317127 abstract "Significance Supported metal nanoparticles often exhibit properties differing from those of their single-crystal counterparts. There have been several suggested explanations for this, including quantum size effects, strong metal support interactions, and some interplay between facets. In this article, we show that the support morphology can also have a decisive role in the nanoparticle properties. Using scanning tunneling microscopy, we show that Pd nanocrystals formed across steps of a TiO 2 support have a curved top facet, where unusual adsorption behavior of CO is found. Calculations suggest that the different adsorption behavior arises from strain originating in the curved top facet. Our observations open the way for the tailoring of nanoparticle functionality by tuning the morphology of the support." @default.
- W1890317127 created "2016-06-24" @default.
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- W1890317127 date "2015-06-15" @default.
- W1890317127 modified "2023-10-12" @default.
- W1890317127 title "Influence of support morphology on the bonding of molecules to nanoparticles" @default.
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- W1890317127 doi "https://doi.org/10.1073/pnas.1506939112" @default.
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