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• W1893773386 abstract "We probe charge photogeneration and subsequent recombination dynamics in neat regioregular poly(3-hexylthiophene) films over six decades in time by means of time-resolved photoluminescence spectroscopy. Exciton dissociation at 10 K occurs extrinsically at interfaces between molecularly ordered and disordered domains. Polaron pairs thus produced recombine by tunneling with distributed rates governed by the distribution of electron-hole radii. Quantum-chemical calculations suggest that hot-exciton dissociation at such interfaces results from a high charge-transfer character." @default.
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• W1893773386 date "2011-05-13" @default.
• W1893773386 modified "2023-10-17" @default.
• W1893773386 title "Charge Separation in Semicrystalline Polymeric Semiconductors by Photoexcitation: Is the Mechanism Intrinsic or Extrinsic?" @default.
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• W1893773386 doi "https://doi.org/10.1103/physrevlett.106.197401" @default.
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