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- W1895320222 abstract "Abstract Measurements of carbonyl sulfide (OCS) have been proposed to provide a unique constraint on carbon assimilation by the biosphere that is independent of the influence of plant and soil respiration of CO 2 , but this constraint depends on a comprehensive understanding of the processes controlling OCS in the biosphere. We conducted a high‐resolution temporal and spatial survey of OCS and CO 2 mixing ratios during the California Nexus Experiment research cruise along the coast of California (U.S.) and into the Sacramento River Delta using a newly constructed compact quantum cascade laser spectrometer (precision for OCS of <8 pptv (pmol/mol) at 1 Hz). The temporal and spatial resolution of the measurements revealed a number of specific processes related to known sources and sinks. The observations demonstrate OCS uptake during daytime photosynthetic uptake of CO 2 , OCS depletion during nighttime forest respiration of CO 2 , and OCS emission from a freshwater marsh. OCS emission was observed in one anthropogenically influenced plume, but, overall, no correlation was observed between OCS and SO 2 , and the use of scaled SO 2 emission fields in global budgets of OCS should be reconsidered for areas with strict sulfur emission controls, such as California. The observations show that, in a homogeneous ecosystem on a local scale, OCS may be a proxy for CO 2 uptake. However, at larger scales that span heterogeneous environments, in order to confidently quantify any single process, competing processes must be either relatively small or well quantified." @default.
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- W1895320222 date "2013-07-22" @default.
- W1895320222 modified "2023-10-15" @default.
- W1895320222 title "Carbonyl sulfide in the planetary boundary layer: Coastal and continental influences" @default.
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- W1895320222 doi "https://doi.org/10.1002/jgrd.50581" @default.
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