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• W1900534651 startingPage "536" @default.
• W1900534651 abstract "As a typical moderately-brominated diphenylethers, 2,2',4,4'-tetrabromodiphenyl ether (BDE47) is hardly debrominated by a conventional TiO2-mediated photocatalysis. However, its reductive debromination was rapid achieved over silver nanoparticle-loaded TiO2 (Ag/TiO2) in UV-irradiated anoxic acetonitrile-water within 13 min. An Ag-promoted electron transfer and C-Br cleavage concept was proposed based on experimental results and density functional theory calculations. Ag(0) exerted affinity interaction with bromine atoms, and the storing of electrons on Ag(0) increased the binding interaction, which elongated the C-Br bond of BDE47 and facilitated its cleavage. The initiating of the BDE47 debromination on Ag(0) required an induction period to enrich a critical amount of electrons, leading to a stronger driving force for both injecting electron to BDE47 and stretching the C-Br bond. Stronger photo-excitation, higher polar solvent, and a moderate Ag(0) load strengthened the interfacial electron transfer over Ag/TiO2, and thereby shortening the induction time and accelerating the BDE47 degradation." @default.
• W1900534651 created "2016-06-24" @default.
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• W1900534651 date "2016-05-01" @default.
• W1900534651 modified "2023-10-09" @default.
• W1900534651 title "Peculiar and rapid photocatalytic degradation of tetrabromodiphenyl ethers over Ag/TiO2 induced by interaction between silver nanoparticles and bromine atoms in the target" @default.
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• W1900534651 doi "https://doi.org/10.1016/j.chemosphere.2015.10.048" @default.
• W1900534651 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26546118" @default.
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