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- W1910040313 abstract "The complex formation between copper(I) ions and glycylglycylglycine (H 2 A + ) has been studied in 3.0 M NaClO 4 medium at 25° by constant current coulometry using copper amalgam and glass electrodes. In each series of measurements the copper ions were generated into the ligand solution by electrolysis of two phases copper amalgam. The data, shown in Table 2, were treated by graphical methods and by the least squares computer program, Letagrop. It is concluded that the results obtained are consistent by assuming the equilibria Cu + + Cu 2+ + 2A − ⇄ Cu I Cu II H –3 A 2 2− + 3H + , log β 11–32 =–3.35 ± 0.04 Cu + + A − ⇄ Cu I A, log β 1001 = 6.2 ± 0.1 where β is an equilibrium constant. It is assumed that the copper(II)‐equilibria, reported in the previous paper of this series, coexist in solution. On the basis of the equilibrium constants it may be deduced that for pH higher than 6.5 the principal copper(I) complex is Cu I Cu II H –3 A 2 2− . The standard oxidation–reduction potential at pH 7 for the formation of this species from its copper(II) analogue, Cu 2 H –4 A 2 2− , was calculated to be +340 mV." @default.
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- W1910040313 date "1970-04-01" @default.
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- W1910040313 title "The Metal Complexes of Peptides and Related Compounds. A Mixed Copper(I)-Copper(II) Complex of Glycylglycylglycine" @default.
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- W1910040313 doi "https://doi.org/10.1111/j.1432-1033.1970.tb00952.x" @default.
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