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- W1914507650 abstract "Atomic crystal structure affects the electromagnetic and thermal properties of common matter. Similarly, the nanoscale structure controls the properties of higher length-scale metamaterials, for example, nanoparticle superlattices and photonic crystals. Electrostatic self-assembly of oppositely charged nanoparticles has recently become a convenient way to produce crystalline nanostructures. However, understanding and controlling the assembly of soft nonmetallic particle crystals with long-range translational order remains a major challenge. Here, we show the electrostatic self-assembly of binary soft particle cocrystals, consisting of apoferritin protein cages and poly(amidoamine) dendrimers (PAMAM), with very large crystal domain sizes. A systematic series of PAMAM dendrimers with generations from two to seven were used to produce the crystals, which showed a dendrimer generation dependency on the crystal structure and lattice constant. The systematic approach presented here offers a transition from trial-and-error experiments to a fundamental understanding and control over the nanostructure. The structure and stability of soft particle cocrystals are of major relevance for applications where a high degree of structural control is required, for example, protein-based mesoporous materials, nanoscale multicompartments, and metamaterials." @default.
- W1914507650 created "2016-06-24" @default.
- W1914507650 creator A5026210883 @default.
- W1914507650 creator A5037006229 @default.
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- W1914507650 date "2015-10-28" @default.
- W1914507650 modified "2023-10-17" @default.
- W1914507650 title "Electrostatic Self-Assembly of Soft Matter Nanoparticle Cocrystals with Tunable Lattice Parameters" @default.
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- W1914507650 doi "https://doi.org/10.1021/acsnano.5b04912" @default.
- W1914507650 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26497975" @default.
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