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- W1920778941 abstract "Abstract The electron donor 2‐isopropylidene‐1,3‐dithiolo[4,5‐ d ]‐4,5‐ethylenediselenotetrathiafulvalene ( 3 ) provides two new molecular conductors, ( 3 ) 2 [M(CN) 2 ] (M = Ag and Au). These salts crystallize in the triclinic P $bar {1}$ space group. The donor sheet structure of these salts is the so‐called β‐type molecular array, in which the donor molecules form a head‐to‐tail dimer. The formation of considerable dimerization and the 2:1 donor–anion ratio result in an effectively half‐filled electronic nature. These salts show metallic conducting behavior from room temperature. The metallic conducting behavior of ( 3 ) 2 [Ag(CN) 2 ] was retained down to 8 K; however, the resistivity of ( 3 ) 2 [Au(CN) 2 ] increased at around 50 K. The magnetic susceptibility of ( 3 ) 2 [Au(CN) 2 ] suggests that the strength of the electron correlation for this salt is enhanced below 50 K." @default.
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- W1920778941 date "2014-04-10" @default.
- W1920778941 modified "2023-09-25" @default.
- W1920778941 title "Molecular Conductors with Effectively Half‐Filled Electronic States Based on Tetrathiafulvalene Derivatives Condensed with a 2‐Isopropylidene‐1,3‐dithiole Ring" @default.
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- W1920778941 doi "https://doi.org/10.1002/ejic.201402006" @default.
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