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• W1920977371 abstract "Although many approaches have been employed to enhance thermal stability of PVA, developing a facile and effective strategy remains highly attractive. Herein, we demonstrate a highly effective approach to strikingly improve thermal stability of PVA by selecting the types of multiamines molecules to tune the hydrogen-bond crosslink density. Results show that only adding 0.5 wt% of 2,4,5,6-tetraaminopyrimidine can make the initial degradation temperature (Ti) and maximum degradation temperature (Tmax) of PVA increase by ∼55 °C and 98 °C due to the formation of 3D physically H-bond crosslinked network, resulting in superior thermal stability property to those of PVA nanocomposites. Moreover, thermal stability strongly depends on the H-bond crosslink density, and Ti and Tmax basically obey the linear hydrogen-bond relations despite some deviations. This work opens up a novel biological methodology for creating thermally stable polymeric materials." @default.
• W1920977371 created "2016-06-24" @default.
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• W1920977371 date "2015-10-01" @default.
• W1920977371 modified "2023-10-16" @default.
• W1920977371 title "Bioinspired strategy for tuning thermal stability of PVA via hydrogen-bond crosslink" @default.
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• W1920977371 doi "https://doi.org/10.1016/j.compscitech.2015.08.006" @default.
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