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• W1933230178 abstract "The heat capacity of synthetic eskolaite, Cr2O3, and of the synthetic spinels magnesiochromite, MgCr2O4, and chromite, FeCr2O4 were measured from 1.5 K to 340 K. For MgCr2O4, a substantial magnetic contribution to the entropy is revealed by a sharp peak in the heat capacity curve at 12.55 ± 0.05 K, which indicates the transition to antiferromagnetic long-range order. Integration of the heat capacity curve yields a value of 118.3 ± 1.2 J/(mol·K) for the standard entropy at 298.15 K, which is in excellent agreement with that calculated from phase equilibria studies on the reaction MgCr2O4+ SiO2 = Cr2O3 + MgSiO3. The new calorimetric results for Cr2O3 indicate a standard entropy at 298.15 K of 82.8 ± 0.8 J/(mol·K). The measurements for FeCr2O4 show three distinct heat capacity anomalies, one of which (peaking at 36.5 ± 0.2 K) was missed by previous low temperature heat capacity measurements, which only extend down to 53 K. Integration of the heat capacity curve yields a value for the standard entropy at 298.15 K of 152.2 ± 3.0 J/(mol·K) for FeCrO4, some 6 J/ (mol·K) greater than the previous calorimetric value." @default.
• W1933230178 created "2016-06-24" @default.
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• W1933230178 date "2000-11-01" @default.
• W1933230178 modified "2023-10-14" @default.
• W1933230178 title "The heat capacity of MgCr₂O₄, FeCr₂O₄, and Cr₂O₃at low temperatures and derived thermodynamic properties" @default.
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• W1933230178 doi "https://doi.org/10.2138/am-2000-11-1212" @default.
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