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• W1943662318 abstract "The prevailing treatment of secondary organic aerosol formation in atmospheric models is based on the assumption of instantaneous gas-particle equilibrium for the condensing species, yet compelling experimental evidence indicates that organic aerosols can exhibit the properties of highly viscous, semisolid particles, for which gas-particle equilibrium may be achieved slowly. The approach to gas-particle equilibrium partitioning is controlled by gas-phase diffusion, interfacial transport, and particle-phase diffusion. Here we evaluate the controlling processes and the time scale to achieve gas-particle equilibrium as a function of the volatility of the condensing species, its surface accommodation coefficient, and its particle-phase diffusivity. For particles in the size range of typical atmospheric organic aerosols (∼50-500 nm), the time scale to establish gas-particle equilibrium is generally governed either by interfacial accommodation or particle-phase diffusion. The rate of approach to equilibrium varies, depending on whether the bulk vapor concentration is constant, typical of an open system, or decreasing as a result of condensation into the particles, typical of a closed system." @default.
• W1943662318 created "2016-06-24" @default.
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• W1943662318 date "2015-09-17" @default.
• W1943662318 modified "2023-10-16" @default.
• W1943662318 title "Under What Conditions Can Equilibrium Gas–Particle Partitioning Be Expected to Hold in the Atmosphere?" @default.
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• W1943662318 doi "https://doi.org/10.1021/acs.est.5b02587" @default.
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