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- W1946394423 abstract "Bioinspired artificial water channels aim to combine the high permeability and selectivity of biological aquaporin (AQP) water channels with chemical stability. Here, we carefully characterized a class of artificial water channels, peptide-appended pillar[5]arenes (PAPs). The average single-channel osmotic water permeability for PAPs is 1.0(± 0.3) × 10(-14) cm(3)/s or 3.5(± 1.0) × 10(8) water molecules per s, which is in the range of AQPs (3.4 ∼ 40.3 × 10(8) water molecules per s) and their current synthetic analogs, carbon nanotubes (CNTs, 9.0 × 10(8) water molecules per s). This permeability is an order of magnitude higher than first-generation artificial water channels (20 to ∼ 10(7) water molecules per s). Furthermore, within lipid bilayers, PAP channels can self-assemble into 2D arrays. Relevant to permeable membrane design, the pore density of PAP channel arrays (∼ 2.6 × 10(5) pores per μm(2)) is two orders of magnitude higher than that of CNT membranes (0.1 ∼ 2.5 × 10(3) pores per μm(2)). PAP channels thus combine the advantages of biological channels and CNTs and improve upon them through their relatively simple synthesis, chemical stability, and propensity to form arrays." @default.
- W1946394423 created "2016-06-24" @default.
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- W1946394423 date "2015-07-27" @default.
- W1946394423 modified "2023-10-14" @default.
- W1946394423 title "Highly permeable artificial water channels that can self-assemble into two-dimensional arrays" @default.
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- W1946394423 doi "https://doi.org/10.1073/pnas.1508575112" @default.
- W1946394423 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4538642" @default.
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