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• W1954264233 abstract "The ion–molecule reactions of the rhenium oxide anions, [ReO x ] − ( x = 2–4) with the organic substrates methane, ethene, methanol, and acetic acid have been examined in a linear ion trap mass spectrometer. The only reactivity observed was between [ReO 2 ] − and acetic acid. Isotope-labelled experiments and high-resolution mass spectrometry measurements were used to assign the formulas of the ionic products. Collision-induced dissociation and ion–molecule reactions with acetic acid were used to probe the structures of the mass-selected primary product ions. Density functional theory calculations [PBE0/LanL2DZ6-311+G(d)] were used to suggest possible structures. The three primary product channels observed are likely to arise from the formation of the metallalactone [ReO 2 (CH 2 CO 2 )] − ( m/z 277) and H 2 , [CH 3 ReO 2 (OH)] − ( m/z 251) and CO, and [ReO 3 ] − ( m/z 235), H 2 and CH 2 CO." @default.
• W1954264233 created "2016-06-24" @default.
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• W1954264233 date "2015-06-01" @default.
• W1954264233 modified "2023-10-10" @default.
• W1954264233 title "Gas-Phase Reactions of the Rhenium Oxide Anions, [ReO_<i>x</i>]⁻ (<i>x</i> = 2–4) with the Neutral Organic Substrates Methane, Ethene, Methanol and Acetic Acid" @default.
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• W1954264233 doi "https://doi.org/10.1255/ejms.1332" @default.
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