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• W1955095680 abstract "Relaxation dynamics of an exclusively adsorbed water molecule in mesoporous silica MCM-41-S was studied by using terahertz spectroscopy. With the temperature controlled from 0 to 50 °C, we observed strongly frequency- and temperature-dependent dielectric relaxation responses, implying that, unlike ice, surface-adsorbed water molecules retained flourishing picosecond dynamics. Based on the Debye relaxation model, a relaxation time constant was found to increase from 1.77 to 4.83 ps when the water molecule was cooled from 50 to 0 °C. An activation energy of ∼15 kJ/mol, which was in close agreement with a hydrogen-bonding energy, was further extracted from the Arrhenius analysis. Combined with previous molecular dynamics simulations, our results indicate that the reorientation relaxation originated from the “flip-flop” rotation of a three hydrogen-bonded surface-adsorbed water molecule." @default.
• W1955095680 created "2016-06-24" @default.
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• W1955095680 date "2015-08-24" @default.
• W1955095680 modified "2023-09-27" @default.
• W1955095680 title "Relaxation dynamics of surface-adsorbed water molecules in nanoporous silica probed by terahertz spectroscopy" @default.
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• W1955095680 doi "https://doi.org/10.1063/1.4929767" @default.
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