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- W1955651419 endingPage "11966" @default.
- W1955651419 startingPage "11960" @default.
- W1955651419 abstract "The nucleation mechanism of water (heterogeneous/homogeneous) can be regulated by confinement within nanoporous alumina. The kinetics of ice nucleation is studied in confinement by employing dielectric permittivity as a probe. Both heterogeneous and homogeneous nucleation, obtained at low and high undercooling, respectively, are stochastic in nature. The temperature interval of metastability extends over ∼4 and 0.4 °C for heterogeneous and homogeneous nucleation, respectively. Nucleation within a pore is spread to all pores in the template. We have examined a possible coupling of all pores through a heat wave and a sound wave, with the latter being a more realistic scenario. In addition, dielectric spectroscopy indicates that prior to crystallization undercooled water molecules relax with an activation energy of ∼50 kJ/mol, and this process acts as precursor to ice nucleation." @default.
- W1955651419 created "2016-06-24" @default.
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- W1955651419 creator A5039070558 @default.
- W1955651419 creator A5042098091 @default.
- W1955651419 creator A5062213262 @default.
- W1955651419 date "2015-08-12" @default.
- W1955651419 modified "2023-09-25" @default.
- W1955651419 title "Kinetics of Ice Nucleation Confined in Nanoporous Alumina" @default.
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- W1955651419 doi "https://doi.org/10.1021/acs.jpcb.5b06295" @default.
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