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- W1963552522 abstract "Abstract Synchrotron radiation photoemission from the Ni 3p and I 4d core levels has been studied for iodine adsorbed on Ni{100} in a range of different phases. In the range of chemisorbed structures involving overlayer compression from coverages θ of about 0.3 to 0.4 the I 4d photoemission binding energies decrease by ~0.3 eV, while further compression to a c(2 × 2) structure leads to a further decrease by ~0.4 eV. Low temperature adsorption of molecular iodine shows a binding energy of 0.1 eV lower still. In the chemisorbed coverage range these core level shifts are found to be substantially less than the I-I repulsive energy interactions and are associated with the through-metal component of this interaction, while the residual component concealed from the photoemission experiments is attributed to through-space overlap interaction. Other processes which may contribute to the observed binding energy shifts, including Coulomb interactions in both initial and final states, are discussed in some detail." @default.
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- W1963552522 date "1984-01-01" @default.
- W1963552522 modified "2023-10-16" @default.
- W1963552522 title "Core level photoemission study of the adsorption of iodine on Ni{100}" @default.
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- W1963552522 doi "https://doi.org/10.1016/0039-6028(84)90653-8" @default.
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